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AV1 playback in LibreELEC on a Pi 4
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Get active cooling as this kinda sounds like thermal throttling.
I added a 40mm Noctua fan blowing on the heatsinks of my pi3 to get it to play h265, otherwise I'd keep having issues like what you're describing.
That's probably the cheapest option. I already have it overclocked and it's running at about 82-83°C (But at 85°C it resets to the base clock so maybe the overclock isn't even being used). Adding active cooling might also allow me to overclock it further.